PySide: Creating GUIs with Qt Creator/Qt Designer or by code?
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I found tutorials that show you 2 different ways to do this:
Using Python, Import PySide
You can create the GUIs directly from a python script, just import PySide and follow the tutorials on this page: http://qt-project.org/wiki/PySideDocumentationUsing QtCreator, PySide and PySide Tools
You can also create the GUI in QtCreator and convert it to a python script. Follow this tutorial:
http://qt-project.org/wiki/QtCreator_and_PySide